Arundel is a town in York County, Maine, United States. At the 2020 census, the population was 4,264. It is part of the Portland–South Portland–Biddeford, Maine Metropolitan Statistical Area. The Municip…Arundel is a town in York County, Maine, United States. At the 2020 census, the population was 4,264. It is part of the Portland–South Portland–Biddeford, Maine Metropolitan Statistical Area. The Municipality of Arundel includes the constituent communities and neighbourhoods of: Arundel Village, Vinegar Hill, Riverside Arundel, Log Cabin Crossing, Goff Mill, Millers Crossing, and Cottagehill, among other neighbourhoods in an inland area adjacent to the Towns of Kennebunkport and Biddeford. In 2014, Arundel was named “Best Place to Live in Maine” by Downeast Magazine.
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