Purcellville is a town in Loudoun County, Virginia. The population was 8,929 according to the 2020 Census. Purcellville is the major population center for Western Loudoun and the Loudoun Valley. M…Purcellville is a town in Loudoun County, Virginia. The population was 8,929 according to the 2020 Census. Purcellville is the major population center for Western Loudoun and the Loudoun Valley. Many of the older structures remaining in Purcellville reflect the Victorian architecture popular during the early twentieth century.
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